ORCID Identifier(s)

ORCID 0000-0002-4259-4172

Graduation Semester and Year

Fall 2024

Language

English

Document Type

Dissertation

Degree Name

Doctor of Philosophy in Materials Science and Engineering

Department

Materials Science and Engineering

First Advisor

Efstathios I. Meletis

Abstract

EPP is an innovative surface modification technique that enables the deposition of metal ions from the electrolyte and their integration with substrate atoms to form intermetallic compound surface layers. EPP offers advantages such as high deposition rates, environmental cleanliness, and operational simplicity. In this study, Ni-Ti intermetallic layers were successfully synthesized on a Ti-6Al-4V substrate using EPP. The properties of the resulting Ni-Ti intermetallic layers were characterized using SEM, EDS, XRD, TEM, nanoindentation, and tribology tests.

This work aims to understand the fabrication mechanism and investigate the effects of various processing parameters on the EPP process. Key factors such as electrolyte concentration, working voltage, processing time, working distance, working temperature, additives, and the amplitude and frequency of the power supply were systematically adjusted to optimize the EPP process. These parameters influence the phase formation, deposition rate, intermetallic layer thickness, and coating coverage of the synthesized intermetallic layers.

Based on the findings, this study demonstrates that EPP is capable of producing various Ti-Ni intermetallic phases at the top surface layer that if desired, can also be followed by a pure Ni top layer. Key EPP processing parameters were identified that control the composition, thickness, uniformity, and surface morphology of the intermetallic phases. A significant enhancement of the tribological properties of Ti-6Al-4V was accomplished by the presence of the intermetallic surface layer. Surface modification via EPP processing resulted in a 148.25% increase in hardness, an 86.43% reduction in wear rate, and a 31.20% decrease in the coefficient of friction.

Keywords

Electrolytic Plasma Processing, Ti and Ti alloys, Ni-Ti intermetallics, Tribology

Disciplines

Metallurgy | Other Materials Science and Engineering | Tribology

License

Creative Commons Attribution 4.0 International License
This work is licensed under a Creative Commons Attribution 4.0 International License.

Available for download on Tuesday, December 30, 2025

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