ORCID Identifier(s)

0009-0002-4505-2739

Graduation Semester and Year

Fall 2024

Language

English

Document Type

Dissertation

Degree Name

Doctor of Philosophy in Materials Science and Engineering

Department

Materials Science and Engineering

First Advisor

Dr. Meletis Efstathios

Second Advisor

Dr. Cao Ye

Abstract

Plasma electrolytic oxidation (PEO) has been extensively applied in the past to improve the tribological properties of titanium and its alloys allowing their widespread use in industrial applications. However, the complete PEO mechanism of action remains unclear. While there are several mathematical models providing useful insights into the PEO process, they do not fully incorporate the effect of applied potential on the outcomes of PEO. In this work, we develop an experimentally informed computational model by expanding on the dielectric breakdown model. We incorporate experimental data to extract key parameters, exploring the iterative dependency of the oxide thickness and ionic current density to predict the oxide growth at various applied external voltages. The model reproduces the PEO process at different constant voltage conditions and the simulation results for the oxide coating thickness over time are in good agreement with the experimental data, validating the application of Faraday’s law and Pyun and Hong's model in describing the coating growth kinetics for the PEO process.

Keywords

Plasma electrolytic oxidation, Titanium, Curve fitting, Potentiostatic, Oxide growth, Galvanostatic, Constant voltage, Constant current

Disciplines

Metallurgy | Other Materials Science and Engineering | Structural Materials

License

Creative Commons Attribution 4.0 International License
This work is licensed under a Creative Commons Attribution 4.0 International License.

Comments

I want to acknowledge.

Dr. Efstathios "Stathis" I. Meletis
Dr. Ye Cao
Mr. Hunter Pitts
Dr. Yao Ren

National Science Foundation UTA/NU Partnership for Research and Education in Materials (NSF DMR-2122128)

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